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Compared to TePP and you may pentaphenylpyrrole (PPP), both TPM and you may TPM-Cl demonstrated prolonged emission wavelengths. Due to their comparable chemical substances formations, that isn’t possible so you can characteristic the main Stokes move so you can variations in the ability gap between the low singlet happy county (S1) and crushed condition (S0). I hence suggest that the newest reddish emission corresponds to a minimal triplet excited state (T1), that’s below S1. 2, where shape are the same on their regular-state emission spectra, sharing the new a lot of time lifetime functions from each other TPM and you will TPM-Cl. The newest lifetimes of the TPM and you may TPM-Cl crystalline powders try 20.step 1 and you may 8.9 μs, correspondingly (Fig. S3 and Desk S1).

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